Brown carbon from biomass burning imposes strong Arctic warming

Increasing wildfires in a warming climate can reinforce the circum-Arctic warming and further contribute to global warming, forming a concerning feedback loop.

Rapid warming in the Arctic and accelerated glacier and sea ice melting have a huge impact on the global environment. Greenhouse gases, such as carbon dioxide, and black carbon aerosols are well-known warming agents. In contrast, atmospheric, light absorbing brown carbon particles belong to the least understood and most uncertain contributors in the Arctic and surrounding regions. An international group of researchers, led by the Institute of Surface-Earth System Science from Tianjin University, China, and the Max Planck Institute for Chemistry, Mainz, Germany, combined direct observations of atmospheric brown carbon particles during a two-month circum-Arctic cruise with comprehensive global model simulations. Their study shows that light absorbing brown carbon, mainly originating from biomass burning can impose strong warming in the Arctic.

“Identifying the warming agents is key to understanding the Arctic warming and finding potential mitigation solutions,” explains Yafang Cheng who heads the Minerva Research Group of the Max Planck Institute for Chemistry in Mainz. The warming effects of brown carbon particles have either been ignored in climate models or estimated with large uncertainties, ranging from approximately 3 per cent to over 50 per cent relative to the warming effect of black carbon. However, observations of brown carbon in the Arctic are sparse, hindering representative assessment of its warming effect in the circum-Arctic.

Combination of observations from a circum-Arctic cruise and model simulations

The international research group thus measured the light-absorption of water-soluble brown carbon from water extracts of aerosol samples (PM10, particulates with diameter < 10 µm) collected from late July to September 2017 during a circum-Arctic cruise. In order to derive source-specific light absorbing properties of brown carbon the group then combined the measured data with the Community Earth System Model. This is a comprehensive numerical simulation of the Earth system consisting of atmospheric, ocean, ice, land surface, carbon cycle, and other components.

Both observations and modelling showed that water-soluble brown carbon on Arctic warming mainly originates from biomass burning in the mid- to high latitudes of the Northern Hemisphere. The combustion contributes approximately 60% of the warming effect of brown carbon in the arctic region on an annual average. In comparison, fossil fuel combustion accounted for approximately 30% of the total radiative absorption effect. “During the summer months, water soluble brown carbon had an average radiative forcing of approximately 90 mW m-2 and, accordingly, a warming effect of approximately 30% relative to black carbon. And, the water insoluble brown carbons may further increase the overall warming effect,” said Siyao Yue, the first author and postdoctoral researcher in Yafang Cheng’s group. These findings highlight the strong impact of biomass burning on Arctic warming, especially in the summertime when Arctic ice melting is most sensitive to the warming.

As climate change is projected to increase the frequency, intensity and spread of wildfires, which in turn will reinforce the arctic warming and further contribute to global warming, forming a positive feedback. “We expect an increasing importance of brown carbon in the warming of the circum-arctic in the future.” said Pingqing Fu, professor at the Tianjin University. “Because biomass burning is also a major source of black carbon, our results highlight the importance of managing vegetation fires, especially in the mid- to high latitudes of the Northern Hemisphere, to mitigate the warming in the Arctic region,” added Yafang Cheng.

Original Publication:
Brown Carbon from Biomass Burning Imposes Strong Circum-Arctic Warming
Siyao Yue1,2,3†, Jialei Zhu1†, Shuang Chen1, Qiaorong Xie1, Wei Li4, Linjie Li3‡, Hong
Ren1,3, Sihui Su1, Ping Li3, Hao Ma1, Yanbing Fan1, Borong Cheng1, Libin Wu1, Jun-jun Deng1, Wei Hu1, Lujie Ren1, Lianfang Wei3, Wanyu Zhao3, Yu Tian3, Xiaole Pan3, Yele Sun3, Zifa Wang3, Fengchang Wu5, Cong-Qiang Liu1, Hang Su6, Joyce E. Penner7, Ulrich Pöschl6, Meinrat O. Andreae6,8, Yafang Cheng2,9*, Pingqing Fu1,3,10*
https://doi.org/10.5281/zenodo.6060

Institutes involved:
1. Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
2. Minerva Research Group, Max Planck Institute for Chemistry, Mainz 55128, Germany
3. State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
4. Third Institute of Oceanography, Ministry of Natural Resources, Xiamen 361005, China
5. State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China
6. Multiphase Chemistry Department, Max Planck Institute for Chemistry, Mainz 55128, Germany
7. Department of Climate and Space Sciences and Engineering, University of Michigan, Ann Arbor, Michigan 48109, USA
8. Department of Geology and Geophysics, King Saud University, Riyadh 11451, Saudi Arabia
9. Department of Precision Machinery and Precision Instrumentation, University of Science and Technology of China, Hefei 230026, China

† These authors contributed equally to this work.
‡ Now at Department of Chemistry and Molecular Biology, University of Gothenburg, Gothenburg, Sweden

Wissenschaftliche Ansprechpartner:

Prof. Dr. Yafang Cheng
E-mail: yafang.cheng@mpic.de
Prof. Dr. Pingqing Fu
E-mail: fupingqing@tju.edu.cn

Originalpublikation:

Brown Carbon from Biomass Burning Imposes Strong Circum-Arctic Warming
Siyao Yue1,2,3†, Jialei Zhu1†, Shuang Chen1, Qiaorong Xie1, Wei Li4, Linjie Li3‡, Hong
Ren1,3, Sihui Su1, Ping Li3, Hao Ma1, Yanbing Fan1, Borong Cheng1, Libin Wu1, Jun-jun Deng1, Wei Hu1, Lujie Ren1, Lianfang Wei3, Wanyu Zhao3, Yu Tian3, Xiaole Pan3, Yele Sun3, Zifa Wang3, Fengchang Wu5, Cong-Qiang Liu1, Hang Su6, Joyce E. Penner7, Ulrich Pöschl6, Meinrat O. Andreae6,8, Yafang Cheng2,9*, Pingqing Fu1,3,10*
https://doi.org/10.5281/zenodo.6060

Weitere Informationen:

https://www.mpic.de/5174411/brown-carbon-arctic-warming?c=3538502