Nanoquakes probe new 2-dimensional material

In a step towards a post-graphene era of new materials for electronic applications, an international team of researchers, including scientists at the University of California, Riverside, has found a new and exciting way to elucidate the properties of novel two-dimensional semiconductors. These materials have unique properties that promise better integration of optical communication with traditional silicon-based devices.

The researchers fabricated a single-atomic-layer-thin film of molybdenum disulfide (MoS₂) on a substrate of lithium niobate (LiNbO₃). LiNbO₃ is used in many electronic devices dealing with high-frequency signals such as cell phones or radar installations. Applying electrical pulses to LiNbO₃, the researchers created very high frequency sound waves – “surface acoustic waves” – that run along the surface of LiNbO₃, akin to earthquake tremors on land. Cell phones, for example, use resonances of these surface waves to filter electric signals in a manner similar to a wine glass resonating when a voice hits it at exactly the right pitch.

Specifically, the research team used the surface waves of LiNbO₃ to listen to how the illumination of LiNbO₃ by laser light changes the electric properties of MoS₂.

“The tone at which a wine glass resonates changes as you fill it up. If you ping it with a spoon, you can hear that tone. With practice you can guess from the tone how full the wine glass is without looking at the glass,” explained Ludwig Bartels, a professor of chemistry who led the team at UC Riverside. “In a similar way, we can 'hear' the LiNbO₃ sound waves and infer how much current the laser light allowed to flow in the MoS₂. We also fabricated transistor structures onto the MoS₂ films and proved that indeed our analysis is correct.”

Study results appeared online last week in Nature Communications.

“The well-established nature of the substrates and the processes to create surface acoustic waves makes the novel technique facile and ready to be applied,” Bartels said. “In particular, even remote, wireless sensing applications appear to be within reach.”

The research project resulted from collaboration between students and researchers at UC Riverside and the University of Augsburg, Germany.

For this project, Bartels's lab greatly benefited from the complementary expertise between the two universities, allowing the researchers to explore new perspectives. Material fabrication proceeded at UCR in Bartels's lab, followed by device integration in Bavaria.

“It was really exciting to see how our students obtained these fascinating results by combining the 2D materials from California and our expertise in surface acoustic waves,” said Hubert Krenner, a member of the Cluster of Excellence Nanosystems Initiative Munich (NIM), Germany, who led the project at the University of Augsburg together with Achim Wixforth. UCR graduate student Edwin Preciado and University of Augsburg recent graduate Florian J. R. Schülein spearheaded the research project in the research laboratories of Bartels and Krenner, respectively.

“International collaboration and my being able to do research work in Germany was crucial for the success of this project,” Preciado said. “I learned much by staying for a few months in Augsburg. It provided me with experience and skills that otherwise I would not have been able to acquire easily.”

Likewise, Sebastian Hammer, a graduate student at the University of Augsburg, worked in Bartels's lab this summer fabricating a new batch of devices in an extension of the current project.

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The research was supported by C-SPIN, a STARnet center of the Semiconductor Research Corporation, the U.S. National Science Foundation, the Deutsche Forschungsgemeinschaft and NIM. The collaborative interaction was facilitated by generous support from the Bavaria-California Technology Center.

Bartels, Krenner, Preciado, Schülein, Hammer and Wixforth were joined in the research by Ariana E. Nguyen, David Barroso, Miguel Isarraraz, Gretel von Son Palacio, I-Hsi Lu and Velveth Klee at UCR; Wladislaw Michailow and Benjamin Moller at the University of Augsburg; and John Mann a recent UCR graduate and now a faculty member at Pepperdine University, Calif.

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